Magnetic dilution in the triangular lattice antiferromagnet NaYb$_{1-x}$Lu$_{x}$O$_2$
Magnetic dilution in the triangular lattice antiferromagnet NaYb$_{1-x}$Lu$_{x}$O$_2$
The delafossite-like compound NaYbO$_2$ hosts a triangular lattice of Yb$^{3+}$ moments and is a promising candidate for realizing a quantum spin liquid state. Here we leverage the substitution of nonmagnetic Lu$^{3+}$ onto the Yb$^{3+}$ sites to track the evolution of the quantum disordered ground state with increasing magnetic disorder in NaYb$_{1-x}$Lu$_x$O$_2$. Low temperature $μ$SR measurements preclude conventional spin freezing and magnetic inhomogeneity, and instead resolve resilient, correlated magnetic fluctuations that persist to at least 15$\%$ dilution. Heat capacity and magnetic susceptibility measurements resolve a rapid suppression of the field-induced ``up-up-down" phase upon introducing magnetic disorder and a crossover in the power-law behavior of the low-temperature magnetic excitations associated with the zero-field quantum disordered ground state. Our combined results place constraints on theories modeling the emergence of the quantum spin liquid-like behavior in NaYbO$_2$.
Steven J. Gomez Alvarado、Brenden R. Ortiz、Soren Bear、Benito A. Gonzalez、Andrea N. Capa Salinas、Adam Berlie、Michael J. Graf、Stephen D. Wilson
物理学
Steven J. Gomez Alvarado,Brenden R. Ortiz,Soren Bear,Benito A. Gonzalez,Andrea N. Capa Salinas,Adam Berlie,Michael J. Graf,Stephen D. Wilson.Magnetic dilution in the triangular lattice antiferromagnet NaYb$_{1-x}$Lu$_{x}$O$_2$[EB/OL].(2025-06-27)[2025-07-20].https://arxiv.org/abs/2506.22613.点此复制
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