低能高电荷态重离子辐照金刚石制备NV色心研究
Production of Nitrogen-Vacancy Color Centers in Diamond Induced by Low Energy Highly Charged Heavy Ion
金刚石中的氮空位(NV)色心因其优异的量子相干性和室温稳定性在量子信息、量子传感等领域具有重要的科学意义和应用价值。本研究利用2.97 MeV的Ar11+高电荷态离子,结合高温退火过程,开展了金刚石NV色心的制备研究。研究发现,在1×1014 ions/cm2离子注量下,辐照和退火处理显著提升了高温高压金刚石样品中NV色心的产额,而1×1015 ions/cm2辐照注量会严重破坏金刚石的晶格结构,造成本底NV色心的显著降低。结果表明,高电荷态重离子辐照可用于精确调控金刚石中NV色心的浓度,退火温度和时长对于提升色心产额有重要作用。本工作还研究了NV色心带隙对温度的依赖性以及高电荷态重离子在材料中的电荷交换过程。这些工作为优化离子辐照制备NV色心技术提供了实验和理论支撑。
he nitrogen vacancy (NV) color center in diamond is of great significance in quantum information and quantum sensing because of its excellent quantum coherence quality and stability at room temperature. In this work, the production of NV color center in diamond was investigated by 2.97 MeV Ar11+ highly charged heavy ion irradition combined with the high temperature annealing process. It is found that the yield of NV color center in diamond samples was significantly increased after the irradiation with a fluence of 11014 ionscm2 and annealing. However, at a higher fluence of 11015 ionscm2, the irradiation seriously destroyed the lattice structure of the diamond, resulting in a significant decrease of the NV color center background. The results show that the concentration of NV color centers in diamond can be precisely controlled by highly charged ion irradiation, and the annealing temperature and duration also play an important role in regulating the color center yield. Furthermore, the dependence of the NV color center band gap on temperature and the charge exchange process of highly charged heavy ions in the material were also studied. These works provide experimental and theoretical support for the optimization of ion irradiation technology for the production of color centers in diamond.
杜广华、张磊、赵灿、郭金龙、毛光博、杜关祥、牟宏进、付林燕
粒子探测技术、辐射探测技术、核仪器仪表物理学半导体技术
金刚石氮空位色心低能高电荷态重离子
diamondnitrogen-vacancy color centerlow energy highly charged heavy ion
杜广华,张磊,赵灿,郭金龙,毛光博,杜关祥,牟宏进,付林燕.低能高电荷态重离子辐照金刚石制备NV色心研究[EB/OL].(2024-12-31)[2025-05-24].https://chinaxiv.org/abs/202412.00395.点此复制
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