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Unified mechanism of charge-density-wave and high-$T_c$ superconductivity protected from oxygen vacancies in bilayer nickelates

Unified mechanism of charge-density-wave and high-$T_c$ superconductivity protected from oxygen vacancies in bilayer nickelates

来源:Arxiv_logoArxiv
英文摘要

Unconventional charge and spin density-wave states are commonly observed in bilayer nickelates, drawing considerable attention due to their proximity to high-$T_c$ superconductivity in various phase diagrams. However, the nature and mechanisms of charge and spin density-waves (DWs) in nickelates remain poorly understood. Numerous experiments have reported that the charge-density-wave (CDW) transition temperature $T_{ cdw}$ and the spin-density-wave (SDW) transition temperature $T_{sdw}$ are closely related but distinct. However, in contrast to these experiments, previous mean-field-type analyses have yielded only a simple SDW phase. To resolve this key problem, this paper demonstrates that sizable CDW instabilities emerge in proportion to the SDW instability in La$3$Ni$2$O$7$.This behavior is driven by the paramagnon-interference (PMI) mechanism, which captures important electron correlations beyond mean-field theory. Therefore, (i) experimental CDW + SDW coexisting state is naturally explained. In addition, (ii) the CDW + SDW fluctuations cooperatively drive high-$T_c$ superconductivity. Notably, the predicted $s$-wave SC state is robust against the inner apical O vacancies. Furthermore, (iii) the CDW instability is highly sensitive to the size of the $d_{z^2}$-orbital hole pocket, allowing for the realization of CDW quantum criticality through carrier-doping and pressure application. We find that the coexistence of charge and spin fluctuations is essential in bilayer nickelates, with both playing a cooperative role in mediating high-$T_c$ superconductivity.

Daisuke Inoue、Youichi Yamakawa、Seiichiro Onari、Hiroshi Kontani

物理学

Daisuke Inoue,Youichi Yamakawa,Seiichiro Onari,Hiroshi Kontani.Unified mechanism of charge-density-wave and high-$T_c$ superconductivity protected from oxygen vacancies in bilayer nickelates[EB/OL].(2025-03-17)[2025-08-02].https://arxiv.org/abs/2503.12925.点此复制

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