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Frequency Dependent Magnetic Susceptibility and the $q^2$ effective conductivity tensor

Frequency Dependent Magnetic Susceptibility and the $q^2$ effective conductivity tensor

来源:Arxiv_logoArxiv
英文摘要

We apply a microscopic formalism for the calculation of material response properties to the problem of the generalization of a first-principles, i.e based on the energy spectrum and geometric properties of the Bloch functions, derivation of the AC magnetic susceptibility. We find that the AC susceptibility forms only a part of the $q^2$ -- where $q$ is the wavevector of the applied field -- effective conductivity tensor, and many additional response tensors characterizing both electric and magnetic multipole moments response to electromagnetic fields and their derivatives must be included to create the full gauge-invariant response. As was seen with the DC magnetic susceptibility and optical activity (characterized by the linear in $q$ contribution to the conductivity) one must be careful with the diagonal elements of the Berry connection. To our knowledge this is the only derivation of such a result general for crystalline insulators, with both `atomic like' contributions and `itinerant contributions' due to overlap of atomic orbitals and non-flat bands. Additionally, quantities familiar from quantum geometry like the Berry connection, curvature, and quantum metric appear extensively.

Alistair H. Duff、J. E. Sipe

物理学

Alistair H. Duff,J. E. Sipe.Frequency Dependent Magnetic Susceptibility and the $q^2$ effective conductivity tensor[EB/OL].(2025-04-02)[2025-07-02].https://arxiv.org/abs/2504.02215.点此复制

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