Room-Temperature Hybrid 2D-3D Quantum Spin System for Enhanced Magnetic Sensing and Many-Body Dynamics

Advances in hybrid quantum systems and their precise control are pivotal for developing advanced quantum technologies. Two-dimensional (2D) materials with optically accessible spin defects have emerged as a promising platform for building integrated quantum spin systems due to their exceptional flexibility and scalability. However, experimentally realizing such systems and demonstrating their superiority remains challenging. Here, we present a hybrid spin system operating under ambient conditions, integrating boron vacancy (VB) spins in 2D hexagonal boron nitride flakes with a single nitrogen vacancy (NV) center in 3D single-crystal diamonds. This combined system achieves full controllability and exhibits enhanced performance for nanoscale magnetic sensing, including an improved dynamic range. Moreover, we investigate the rich many-body spin dynamics within the hybrid system, enabling the first-time quantification of the fluorescence intensity of a single VB defect at 104 counts per second. This result represents a critical step toward the direct optical observation of single VB defects.