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首页|Dominant apical-oxygen electron-phonon coupling in HgBa$_2$Ca$_2$Cu$_3$O$_{8+\delta}$

Dominant apical-oxygen electron-phonon coupling in HgBa$_2$Ca$_2$Cu$_3$O$_{8+\delta}$

Dominant apical-oxygen electron-phonon coupling in HgBa$_2$Ca$_2$Cu$_3$O$_{8+\delta}$

来源:Arxiv_logoArxiv
英文摘要

How electron-phonon interactions influence high-temperature superconductivity in cuprates remains contested, and their role outside the CuO$_2$ planes has been largely overlooked. The most conspicuous evidence for such coupling is the ubiquitous 70-meV dispersion kink seen by photoemission, yet its microscopic origin is still debated. Here we use oxygen-$K$-edge resonant inelastic X-ray scattering (RIXS) to probe the trilayer cuprate HgBa$_2$Ca$_2$Cu$_3$O$_{8+\delta}$ (Hg1223). When both incident photon energy and polarization are tuned to the apical-oxygen $1s\!\rightarrow\!2p_z$ transition, the RIXS spectra exhibit a ladder of at least ten phonon overtones, evenly spaced by 70 meV, whose intensities follow a Franck-Condon envelope, signalling exceptionally strong electron-phonon coupling. Quantitative modelling that incorporates core-hole lifetime evaluation yields an apical-phonon coupling energy of 0.25(1) eV, significantly larger than that of the planar stretching mode. Such a coupling strength offers a strong contender for explaining the universal 70-meV kink and suggests that the dominant electron-phonon channel resides outside the CuO$_2$ planes. By elevating inter-layer lattice dynamics from a peripheral factor to a central actor, our results provide a fresh starting point for theories seeking to reconcile strong correlations, lattice dynamics and high-temperature superconductivity.

Wenshan Hong、Qizhi Li、Shilong Zhang、Qian Xiao、Sahil Tippireddy、Jie Li、Yuchen Gu、Shichi Dong、Taimin Miao、Xiangyu Luo、Xianghong Jin、Lin Zhao、Xingjiang Zhou、Ke-Jin Zhou、Yi Lu、Yingying Peng、Yuan Li

自然科学理论自然科学研究方法电工材料

Wenshan Hong,Qizhi Li,Shilong Zhang,Qian Xiao,Sahil Tippireddy,Jie Li,Yuchen Gu,Shichi Dong,Taimin Miao,Xiangyu Luo,Xianghong Jin,Lin Zhao,Xingjiang Zhou,Ke-Jin Zhou,Yi Lu,Yingying Peng,Yuan Li.Dominant apical-oxygen electron-phonon coupling in HgBa$_2$Ca$_2$Cu$_3$O$_{8+\delta}$[EB/OL].(2025-04-30)[2025-06-22].https://arxiv.org/abs/2505.00223.点此复制

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