Constraints on magnetism and correlations in RuO$_2$ from lattice dynamics and M\"ossbauer spectroscopy
Constraints on magnetism and correlations in RuO$_2$ from lattice dynamics and M\"ossbauer spectroscopy
We provide experimental evidence for the absence of a magnetic moment in bulk RuO$_2$, a candidate altermagnetic material, by using a combination of M\"ossbauer spectroscopy, nuclear forward scattering, inelastic X-ray and neutron scattering, and density functional theory calculations. Using complementary M\"ossbauer and nuclear forward scattering we determine the $^{99}$Ru magnetic hyperfine splitting to be negligible. Inelastic X-ray and neutron scattering derived lattice dynamics of RuO$_2$ are compared to density functional theory calculations of varying flavors. Comparisons among theory with experiments indicate that electronic correlations, rather than magnetic order, are key in describing the lattice dynamics.
George Yumnam、Parul R. Raghuvanshi、John D. Budai、Dipanshu Bansal、Lars Bocklage、Douglas Abernathy、Yongqiang Cheng、Ayman Said、Igor I. Mazin、Haidong Zhou、Benjamin A. Frandsen、David S. Parker、Lucas R. Lindsay、Valentino R. Cooper、Michael E. Manley、Rapha?l P. Hermann
物理学
George Yumnam,Parul R. Raghuvanshi,John D. Budai,Dipanshu Bansal,Lars Bocklage,Douglas Abernathy,Yongqiang Cheng,Ayman Said,Igor I. Mazin,Haidong Zhou,Benjamin A. Frandsen,David S. Parker,Lucas R. Lindsay,Valentino R. Cooper,Michael E. Manley,Rapha?l P. Hermann.Constraints on magnetism and correlations in RuO$_2$ from lattice dynamics and M\"ossbauer spectroscopy[EB/OL].(2025-05-06)[2025-07-16].https://arxiv.org/abs/2505.03250.点此复制
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