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福建省分行业挥发性有机液体储罐VOCs和物种排放清单

中文摘要英文摘要

油气挥发源VOCs排放是区域大气臭氧前体物的重要来源,实现福建省挥发性有机液体储罐VOCs排放精细化管控,本研究基于优化的储罐VOCs排放清单算法,使用逐小时气象观测数据、储罐实际工程参数、物料信息以及物料周转量,综合不同储存物料的源谱,计算福建省高时空分辨率挥发性有机液体储罐VOCs排放清单和物种排放清单。结果表明福建省涉挥发性物料储罐共1886个,其中内浮顶罐870个,固定顶罐950个,外浮顶罐66个,VOCs年排放总量为12022.85±223.2吨,不同物料排放因子为2.96~5.35 吨/ 万吨,其中内浮顶罐排放占比64.4%,油气仓储是主要排放行业(47.5%),主要的排放物种分别是烷烃(7252.4±148.6吨,60.33%)、OVOCs(1861.7±26.2吨,15.49%)和芳香烃(1717.4±26.4吨,14.29%)。在时间分布上,不同月份相对均值波动在667.34~1345.99吨。

Volatile organic compound (VOCs) emissions from oil and gas evaporation sources are a critical precursor to regional atmospheric ozone formation. To achieve refined management of VOCs emissions from volatile organic liquid storage tanks in Fujian Province, this study employs an optimized VOCs emission inventory algorithm, integrating hourly meteorological observation data, actual engineering parameters of storage tanks, material properties, material throughput, and source profiles of stored substances. This approach calculates a high spatiotemporal resolution VOCs emission inventory and species-specific emission inventory for FEmission Inventory of VOCs and Specific Species from Volatile Organic Liquid Storage Tanks in the Storage-Related Industries of Fujian Provinceujian\'s organic liquid storage tanks. The results indicate that Fujian Province has 1,886 storage tanks handling volatile organic materials, including 870 internal floating roof tanks, 950 fixed roof tanks, and 66 external floating roof tanks. The total annual VOCs emissions amount to 12,022.85 ±13.86 tons, with emission factors ranging from 2.96 to 5.35 tons per 10,000 tons of material throughput. Internal floating roof tanks contribute 64.4% of total emissions, and the oil and gas storage sector dominates emissions at 47.5%. The primary emitted species are alkanes (7,252.4 ±9.6 tons, 60.33%), oxygenated volatile organic compounds (OVOCs, 1,861.7 ±3.5 tons, 15.49%), and aromatic hydrocarbons (1,717.4 ±3.0 tons, 14.29%). Temporally, monthly emissions fluctuate between 667.34 and 1,345.99 tons relative to the annual mean.

何宇强、邵晓寒、满瀚阳、倪尔灵、钟雪芬

福建师范大学环境与资源学院,福建省福州市 350117福建师范大学环境与资源学院,福建省福州市 350117福建师范大学环境与资源学院,福建省福州市 350117福建省环境科学研究院,福建省福州市 350013福建省环境科学研究院,福建省福州市 350013

环境污染、环境污染防治石油天然气储运

挥发性有机液体储罐VOCs储罐物种排放

Volatile Organic Liquid Storage TanksVOCsSpeciated from Storage Tanks

何宇强,邵晓寒,满瀚阳,倪尔灵,钟雪芬.福建省分行业挥发性有机液体储罐VOCs和物种排放清单[EB/OL].(2025-05-21)[2025-05-24].http://www.paper.edu.cn/releasepaper/content/202505-130.点此复制

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