Spatial correlations of charge density wave order across the transition in 2H-NbSe2
Spatial correlations of charge density wave order across the transition in 2H-NbSe2
Charge density waves (CDWs) involve coupled amplitude and phase degrees of freedom, but direct access to local amplitude correlations remains experimentally challenging. Here, we report cryogenic four-dimensional scanning transmission electron microscopy (4D-STEM) measurements of CDW ordering in 2H-NbSe2, enabled by liquid helium-based cooling down to 20 K. By mapping the spatial distribution of CDW superlattice intensities at nanometer-scale resolution and analyzing their autocorrelations, we extract the temperature-dependent correlation length associated with the local amplitude of the CDW order parameter, independent of global phase coherence. Our results reveal that weak short-range amplitude correlations persist above the transition temperature, and grow significantly upon cooling, reaching approximately 150 nm at 20 K. These findings demonstrate clear deviations from mean-field expectations and establish 4D-STEM as a powerful tool for probing spatially inhomogeneous electronic order in quantum materials.
Seokjo Hong、Jaewhan Oh、Woohyun Cho、Soyoung Lee、Colin Ophus、Yeongkwan Kim、Heejun Yang、SungBin Lee、Yongsoo Yang
物理学晶体学
Seokjo Hong,Jaewhan Oh,Woohyun Cho,Soyoung Lee,Colin Ophus,Yeongkwan Kim,Heejun Yang,SungBin Lee,Yongsoo Yang.Spatial correlations of charge density wave order across the transition in 2H-NbSe2[EB/OL].(2025-06-03)[2025-06-22].https://arxiv.org/abs/2506.02991.点此复制
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