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Magnetic and thermodynamic studies on the distorted kagome magnet Pr$_3$BWO$_9$

Magnetic and thermodynamic studies on the distorted kagome magnet Pr$_3$BWO$_9$

来源:Arxiv_logoArxiv
英文摘要

We report specific heat, ac/dc magnetic susceptibility as well as static and pulsed field magnetization studies on the distorted kagome magnet Pr$_3$BWO$_9$ down to 0.4~K and up to high magnetic fields. The low-temperature thermodynamic properties are found to be governed by an electronic quasi-doublet ground state; the energy splitting of which amounts to $\Delta_1\simeq 18$ K and exhibits a quadratic field dependence with $g_\mathrm{eff} = 2.6$. Fitting of the specific heat data implies that the next excited state is strongly gapped at $\Delta_2=430$ K and three-fold degenerate in zero field. Our dc and ac susceptibility studies down to 0.4 K do not detect signatures of distinct spin glass behavior. Pulsed field magnetization measurements up to 60 T confirm the Ising-like paramagnetic nature of the magnetic ground state which is characterized by $m_J=\pm 4$ and the anisotropy energy $E_a\simeq 950$ K.

Ahmed Elghandour、Jan Arneth、Annu Yadav、Sven Luther、Panchanan Khuntia、Rüdiger Klingeler

物理学

Ahmed Elghandour,Jan Arneth,Annu Yadav,Sven Luther,Panchanan Khuntia,Rüdiger Klingeler.Magnetic and thermodynamic studies on the distorted kagome magnet Pr$_3$BWO$_9$[EB/OL].(2025-06-06)[2025-07-16].https://arxiv.org/abs/2506.06070.点此复制

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