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Quantum Griffiths phase in the kagome Kondo lattice CeRh$_{0.9}$Pd$_{0.1}$Sn

Quantum Griffiths phase in the kagome Kondo lattice CeRh$_{0.9}$Pd$_{0.1}$Sn

来源:Arxiv_logoArxiv
英文摘要

CeRhSn is a valence fluctuating heavy-fermion metal with a twisted Ce-kagome lattice, displaying zero-field quantum criticality, previously associated with geometrical frustration. The partial substitution of Rh by Pd in CeRh$_{1-x}$Pd$_x$Sn enlarges the unit-cell volume, suppresses valence fluctuations, decreases the Kondo temperature and stabilizes a possible long-range antiferromagnetic (AFM) ordered ground state with $T_N=0.8$ K at $x=0.5$. Previous thermodynamic and spectroscopic measurements for $x=0.1$ suggested a quantum critical spin liquid. We report low-temperature dilatometry and magnetization measurements on CeRh$_{0.9}$Pd$_{0.1}$Sn and compare with published low-$T$ specific heat data. The absence of a Grüneisen parameter divergence excludes a conventional quantum criticality scenario. Instead, the weak power-law divergences signal non-Fermi liquid (NFL) behavior, according to a disorder-driven quantum Griffiths phase scenario. At low temperatures, a negative thermal expansion is found in fields above approximately 0.5 T and the NFL scaling breaks down, probably due to the polarization of AFM correlations.

Nan Tang、Rajesh Tripathi、Yasuyuki Shimura、Toshiro Takabatake、Devashibhai A. Adroja、Philipp Gegenwart

物理学

Nan Tang,Rajesh Tripathi,Yasuyuki Shimura,Toshiro Takabatake,Devashibhai A. Adroja,Philipp Gegenwart.Quantum Griffiths phase in the kagome Kondo lattice CeRh$_{0.9}$Pd$_{0.1}$Sn[EB/OL].(2025-07-24)[2025-08-10].https://arxiv.org/abs/2507.18422.点此复制

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