High-efficiency and broadband coherent optical comb generation in integrated X-cut lithium niobate microresonators

The ability to generate efficient and coherent frequency combs using photonic integrated circuits offers tremendous potential for a range of applications. In particular, "microcombs" based on chip-integrated resonators are poised to revolutionize optical communication, computation, and sensing systems, especially when paired with fast electro-optic (EO) devices. X-cut thin-film lithium niobate (TFLN) is a promising platform for developing the next-generation of microcomb-driven integrated photonic systems, providing a diversity of functionalities through combined $χ^{(3)}$ and EO nonlinearities. In this context, normal-dispersion Kerr microcombs are critically needed because of their standout advantages, yet this dispersion regime remains unexplored for comb generation on X-cut TFLN. Here, we leverage ultralow-loss photonic waveguides, as well as strategic resonator designs that allow us to tailor Raman effects and engineer desired spatial mode interactions, for the robust generation of normal-dispersion Kerr microcombs. Specifically, we show microcombs that substantially surpass state-of-the-art bright cavity soliton and EO microcombs on X-cut TFLN in key performance metrics. Additionally, we demonstrate a novel microcomb whose existence is underpinned by both normal-dispersion Kerr dynamics and stimulated Raman scattering, in a single spatial mode of a microresonator. This microcomb manifests itself as two interleaved frequency combs centered about the pump and Stokes frequencies, resulting in extended spectral spans. Our work will unlock high-speed and low energy consumption photonic circuits for communications, frequency synthesis, and signal processing enabled by a monolithic microcomb technology, while also stimulating further investigations of new nonlinear states that may synergize the strong hybrid nonlinearities unique to X-cut TFLN.