Quantum electrodynamical time-dependent density functional theory on a lattice
Quantum electrodynamical time-dependent density functional theory on a lattice
We present a rigorous formulation of the time-dependent density functional theory for interacting lattice electrons strongly coupled to cavity photons. We start with an example of one particle on a Hubbard dimer coupled to a single photonic mode, which is equivalent to the single mode spin-boson model or the quantum Rabi model. For this system we prove that the electron-photon wave function is a unique functional of the electronic density and the expectation value of the photonic coordinate, provided the initial state and the density satisfy a set of well defined conditions. Then we generalize the formalism to many interacting electrons on a lattice coupled to multiple photonic modes and prove the general mapping theorem. We also show that for a system evolving from the ground state of a lattice Hamiltonian any density with a continuous second time derivative is locally $v$-representable.
Mehdi Farzanehpour、I. V. Tokatly
物理学
Mehdi Farzanehpour,I. V. Tokatly.Quantum electrodynamical time-dependent density functional theory on a lattice[EB/OL].(2014-08-27)[2025-05-15].https://arxiv.org/abs/1408.6324.点此复制
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