利用几个光周期太赫兹脉冲控制耗散环境中分子定向
Nonadiabatically molecular orientation in dissipative environment by THz few-cycle pulses
本文提出利用几个光周期太赫兹脉冲实现耗散环境中分子定向的理论控制方案。通过求解多能级布洛赫模型下的量子刘维尔方程计算得到数值结果。计算结果表明分子定向度对太赫兹脉冲的载波相位比较敏感。计算了耗散环境中的一氧化分子在不同压强和温度下的定向和转动布居。另外,还讨论了纯退相干对分子定向的影响。
We present a theoretical scheme to achieve the nonadiabatically molecular orientation in dissipative environment by THz few-cycle pulses. Numerical calculations are performed by solving the quantum Liouville equation based on multilevel Bloch model. The molecular orientation degree is sensitive to the carrier-envelope phases of the THz pulses. The orientation and the rotational population of CO molecules in dissipative environment (bath) are computed at different pressures and temperatures. The influence of pure decoherence on the molecular orientation is also discussed.
李健、刘勇、于杰、丛书林
物理学
分子定向太赫兹脉冲耗散动力学
Molecular orientationTHz Pulsedissipative dynamics
李健,刘勇,于杰,丛书林.利用几个光周期太赫兹脉冲控制耗散环境中分子定向[EB/OL].(2013-01-04)[2025-08-16].http://www.paper.edu.cn/releasepaper/content/201301-51.点此复制
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