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Graphene-driven correlated electronic states in one dimensional defects within WS$_2$

Graphene-driven correlated electronic states in one dimensional defects within WS$_2$

来源:Arxiv_logoArxiv
英文摘要

Tomonaga-Luttinger liquid (TLL) behavior in one-dimensional systems has been predicted and shown to occur at semiconductor-to-metal transitions within two-dimensional materials. Reports of one-dimensional defects hosting a Fermi liquid or a TLL have suggested a dependence on the underlying substrate, however, unveiling the physical details of electronic contributions from the substrate require cross-correlative investigation. Here, we study TLL formation within defectively engineered WS$_2$ atop graphene, where band structure and the atomic environment is visualized with nano angle-resolved photoelectron spectroscopy, scanning tunneling microscopy and spectroscopy, and non-contact atomic force microscopy. Correlations between the local density of states and electronic band dispersion elucidated the electron transfer from graphene into a TLL hosted by one-dimensional metal (1DM) defects. It appears that the vertical heterostructure with graphene and the induced charge transfer from graphene into the 1DM is critical for the formation of a TLL.

Antonio Rossi、Johannes T. Küchle、Mauricio Terrones、Archana Raja、Adam Schwartzberg、John C. Thomas、Zhuohang Yu、D. Frank Ogletree、Willi Auwärter、Eli Rotenberg、Alexander Weber-Bargioni、Jeffrey B. Neaton、Michael F. Crommie、Francesco Allegretti、Elyse Barré、Da Zhou、Shalini Kumari、Hsin-Zon Tsai、Ed Wong、Chris Jozwiak、Aaron Bostwick、Joshua A. Robinson

10.1038/s41467-025-60993-x

物理学

Antonio Rossi,Johannes T. Küchle,Mauricio Terrones,Archana Raja,Adam Schwartzberg,John C. Thomas,Zhuohang Yu,D. Frank Ogletree,Willi Auwärter,Eli Rotenberg,Alexander Weber-Bargioni,Jeffrey B. Neaton,Michael F. Crommie,Francesco Allegretti,Elyse Barré,Da Zhou,Shalini Kumari,Hsin-Zon Tsai,Ed Wong,Chris Jozwiak,Aaron Bostwick,Joshua A. Robinson.Graphene-driven correlated electronic states in one dimensional defects within WS$_2$[EB/OL].(2025-07-08)[2025-07-22].https://arxiv.org/abs/2301.02721.点此复制

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