低能N+-He 碰撞中的态选择单电子俘获研究
State-selective single electron capture in slow N+-He collisions
利用反应显微成像谱仪,采用二重符合方法,实验测量了0.64 keV/u N<sup>+</sup> 与He 单电子俘获产生的反冲离子He<sup>+</sup> 三维动量,获得了电子俘获到炮弹离子不同量子态的态选择截面和角分布。实验结果表明:基态的 炮弹离子N<sup>+</sup>(1s<sup>2</sup>2s<sup>2</sup>2p<sup>2</sup> <sup>3</sup>P) 俘获He 靶的一个1s 电子主要布居到2p 壳层,也可以看到布居到更高壳层的贡献; 亚稳态的炮弹离子N<sup>+</sup>(1s<sup>2</sup>2s2p<sup>3</sup> <sup>5</sup>S) 俘获He 靶的一个1s 电子主要布居到2s 壳层,几乎看不到布居到更高壳层 的贡献。利用NHe<sup>+</sup> 准分子离子的势能曲线定性地解释了实验结果,但分子库仑过垒模型的反应窗预测与实 验存在较大差别。在亚稳态炮弹离子N<sup>+</sup>(1s<sup>2</sup>2s2p<sup>3</sup> <sup>5</sup>S) 俘获靶电子到2s 轨道的过程中,角微分截面出现了明显 的振荡结构, 这很可能来自Demkov 型跃迁。
he state-selective single-electron capture process in the collision of N<sup>+</sup> ions with He at an energy of 0.64 keV/u has been experimentally studied by the reaction microscopy with a two-fold coincident method, and the state-selective cross-sections and angular distributions of an electron captured into different quantum states of the projectile ions have been obtained. The experimental results show that: the ground state projectile N<sup>+</sup>(<sup>3</sup>P) captures a 1 electron from the He target mainly to the 2 shell, and the contribution to the higher shells can also be observed; the metastable N<sup>+</sup>(<sup>5</sup>S) captures a 1 electron from the He target mainly to the 2 shell, with almost no contribution to higher shells. The experimental results are interpreted qualitatively using the potential energy curves of the NHe<sup>+</sup> quasimolecular ion, but the reaction window predictions of the molecular Coulomb over-barrier model differ significantly from the experiments. During the capture of the target electron into the 2 orbital by the metastable projectile N<sup>+</sup>(<sup>5</sup>S), a clear oscillatory structure appears in the angular differential cross-section, which is likely to result from Demkov-type transitions.
物理学
单电子俘获态选择截面角微分截面亚稳态离子原子碰撞
single-electron capturestate-selective cross-sectionsangular differential cross-sectionsmetastable statesion-atom collisions
.低能N+-He 碰撞中的态选择单电子俘获研究[EB/OL].(2024-02-22)[2025-08-17].https://chinaxiv.org/abs/202402.00226.点此复制
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