|国家预印本平台
首页|Determination of the nearest-neighbor interaction in VO$_2$ via fractal dimension analysis

Determination of the nearest-neighbor interaction in VO$_2$ via fractal dimension analysis

Determination of the nearest-neighbor interaction in VO$_2$ via fractal dimension analysis

来源:Arxiv_logoArxiv
英文摘要

The Ising model is one of the simplest and most well-established concepts to simulate phase transformations in complex materials. However, its most central constant, the interaction strength J between two nearest neighbors, is hard to obtain. Here we show how this basic constant can be determined with a fractal dimension analysis of measured domain structures. We apply this approach to vanadium dioxide, a strongly correlated material with a first-order insulator-to-metal phase-transition with enigmatic properties. We obtain a nearest-neighbor interaction of 13.8 meV, a value close to the thermal energy at room temperature. Consequently, even far below the transition temperature, there are spontaneous local phase-flips from the insulating into the metallic phase. These fluctuations explain several measured anomalies in VO$_2$, in particular the low thermal carrier activation energy and the finite conductivity of the insulating phase. As a method, our fractal dimension analysis links the Ising model to macroscopic material constants for almost any first-order phase transition.

Jacob Holder、Peter Baum、Peter Nielaba、Daniel Kazenwadel

物理学

Jacob Holder,Peter Baum,Peter Nielaba,Daniel Kazenwadel.Determination of the nearest-neighbor interaction in VO$_2$ via fractal dimension analysis[EB/OL].(2023-06-16)[2025-08-02].https://arxiv.org/abs/2306.09722.点此复制

评论